An investigation on the persistence of uranium hydride during storage of simulant nuclear waste packages. (doi:10.7910/DVN/55LJ9P)

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Document Description

Citation

Title:

An investigation on the persistence of uranium hydride during storage of simulant nuclear waste packages.

Identification Number:

doi:10.7910/DVN/55LJ9P

Distributor:

Harvard Dataverse

Date of Distribution:

2015-04-23

Version:

1

Bibliographic Citation:

Stitt, Camilla, 2015, "An investigation on the persistence of uranium hydride during storage of simulant nuclear waste packages.", https://doi.org/10.7910/DVN/55LJ9P, Harvard Dataverse, V1

Study Description

Citation

Title:

An investigation on the persistence of uranium hydride during storage of simulant nuclear waste packages.

Identification Number:

doi:10.7910/DVN/55LJ9P

Authoring Entity:

Stitt, Camilla (University of Bristol)

Distributor:

Harvard Dataverse

Access Authority:

Stitt, Camilla

Depositor:

Stitt, Camilla

Date of Deposit:

2015-04-23

Holdings Information:

https://doi.org/10.7910/DVN/55LJ9P

Study Scope

Keywords:

Physics

Abstract:

Synchrotron X-rays have been used to study the oxidation of uranium and uranium hydride when encapsulated in grout and stored in de-ionised water for 10 months. Periodic synchrotron X-ray tomography and X-ray powder diffraction have allowed measurement and identification of the arising corrosion products and the rates of corrosion. The oxidation rates of the uranium metal and uranium hydride were slower than empirically derived rates previously reported for each reactant in an anoxic water system, but without encapsulation in grout. This was attributed to the grout acting as a physical barrier limiting the access of oxidising species to the uranium surface. Uranium hydride was observed to persist throughout the 10 month storage period and industrial consequences of this observed persistence are discussed.

Notes:

Supplementary and raw data for the article titled 'An investigation on the persistence of uranium hydride during storage of simulant nuclear waste packages.' authored by C. A. Stitt, N. J. Harker, K. R. Hallam, C. Paraskevoulakos, A. Banos, S. Rennie, J. Jowsey, T.B. Scott

Methodology and Processing

Sources Statement

Data Access

Notes:

<a href="http://creativecommons.org/publicdomain/zero/1.0">CC0 1.0</a>

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